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• W2897110526 abstract "Interface failure due to thermal mismatch is one of the culprits that shorten life cycle of devices. In this work, we prepared a series of free-standing cross-linked polyarylamide films with tunable thermal responsive behaviors. By incorporating thermal contractile units, s-dibenzocyclooctadiene (DBCOD), which shrink as a result of thermally induced upconversion from twist boat to chair, negative, zero, and positive coefficients of thermal expansion (CTE) have been realized with the values of CTE ranging from −17.7 to 57.1 ppm/K (20–150 °C). This wide tunable CTE window allows the as-prepared cross-linked polyarylamide films to match desired thermal performance for specific applications. Zero-expansion polymer film without the need for inorganic dopants has also been obtained. Such a series of free-standing polyarylamide films with tunable thermal responses showed great potential for many practical applications." @default.
• W2897110526 created "2018-10-26" @default.
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• W2897110526 date "2018-10-17" @default.
• W2897110526 modified "2023-10-04" @default.
• W2897110526 title "Zero Thermal Expansion Polyarylamide Film with Reversible Conformational Change Structure" @default.
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• W2897110526 doi "https://doi.org/10.1021/acs.macromol.8b01890" @default.
• W2897110526 hasPublicationYear "2018" @default.
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