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• W2897211135 abstract "In this work, we demonstrate a synthetic route to attain methylammonium lead bromide (CH3NH3PbBr3) perovskite nanocrystals (nc-MAPbBr3, 1.5 nm < size < 3 nm) and provide them with functionality as highly efficient flexible, transparent, environmentally stable, and adaptable color-converting films. We use nanoparticle metal oxide (MOx) thin films as porous scaffolds of controlled nanopores size distribution to synthesize nc-MAPbBr3 through the infiltration of perovskite liquid precursors. We find that the control over the reaction volume imposed by the nanoporous scaffold gives rise to a strict control of the nanocrystal size, which allows us to observe well-defined quantum confinement effects on the photo-emission, being the luminescence maximum tunable with precision between λ = 530 nm (green) and λ = 490 nm (blue). This hybrid nc-MAPbBr3/MOx structure presents high mechanical stability and permits subsequent infiltration with an elastomer to achieve a self-standing flexible film, which not only maintains the photo-emission efficiency of the nc-MAPbBr3 unaltered but also prevents their environmental degradation. Applications as adaptable color-converting layers for light-emitting devices are envisaged and demonstrated." @default.
• W2897211135 created "2018-10-26" @default.
• W2897211135 creator A5029583949 @default.
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• W2897211135 date "2018-10-12" @default.
• W2897211135 modified "2023-10-05" @default.
• W2897211135 title "Highly Efficient and Environmentally Stable Flexible Color Converters Based on Confined CH₃NH₃PbBr₃ Nanocrystals" @default.
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• W2897211135 doi "https://doi.org/10.1021/acsami.8b11706" @default.
• W2897211135 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30360096" @default.
• W2897211135 hasPublicationYear "2018" @default.
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