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- W2897383722 abstract "Abstract Electrochemical generation of ammonia (NH 3 ) from nitrogen (N 2 ) using renewable electricity is a desirable alternative to current NH 3 production methods, which consume roughly 1 % of the world's total energy use. The use of catalysts to manipulate the required electron and proton transfer reactions with low energy input is also a chemical challenge that requires development of fundamental reaction pathways. This work presents an approach to the electrochemical reduction of N 2 into NH 3 using a coordination complex of aluminum(III), which facilitates NH 3 production at −1.16 V vs. SCE. Reactions performed under 15 N 2 liberate 15 NH 3 . Electron paramagnetic resonance spectroscopic characterization of a reduced intermediate and investigations of product inhibition, which limit the reaction to sub‐stoichiometric, are also presented." @default.
- W2897383722 created "2018-10-26" @default.
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- W2897383722 date "2018-10-30" @default.
- W2897383722 modified "2023-10-14" @default.
- W2897383722 title "Electrochemical Reduction of N <sub>2</sub> to NH <sub>3</sub> at Low Potential by a Molecular Aluminum Complex" @default.
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- W2897383722 doi "https://doi.org/10.1002/chem.201804454" @default.
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