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• W2897423743 abstract "Spin-orbit (SO) Mott insulators are regarded as a new paradigm of magnetic materials, whose properties are largely influenced by SO coupling and featured by highly anisotropic bond-dependent exchange interactions between the spin-orbital entangled Kramers doublets, as typically manifested in $5d$ iridates. Here, we propose that a very similar situation can be realized in cuprates when the ${mathrm{Cu}}^{2+}$ ions reside in a tetrahedral environment, as in spinel compounds. Using first-principles electronic structure calculations, we construct a realistic model for the diamond lattice of the ${mathrm{Cu}}^{2+}$ ions in ${mathrm{CuAl}}_{2}{mathrm{O}}_{4}$ and show that the magnetic properties of this compound are largely controlled by anisotropic compass-type exchange interactions that dramatically modify the magnetic ground state by lifting the spiral spin-liquid degeneracy and stabilizing a commensurate single-$mathbit{q}$ spiral." @default.
• W2897423743 created "2018-10-26" @default.
• W2897423743 creator A5029910949 @default.
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• W2897423743 date "2018-11-12" @default.
• W2897423743 modified "2023-10-16" @default.
• W2897423743 title "Realization of the anisotropic compass model on the diamond lattice of <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:msup><mml:mrow><mml:mi>Cu</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn><mml:mo>+</mml:mo></mml:mrow></mml:msup></mml:math> in <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:mrow><mml:msub><mml:mi>CuAl</mml:mi><mml:mn>2</mml:mn></mml:msub><mml:msub><mml:mi mathvariant=normal>O</mml:mi><mml:mn>4</mml:mn></mml:msub></mml:mrow></mml:math>" @default.
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• W2897423743 doi "https://doi.org/10.1103/physrevb.98.201106" @default.
• W2897423743 hasPublicationYear "2018" @default.
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