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- W2897428253 abstract "A step-shear deformation imparts an instantaneous, anisotropic stimulus onto a microphase-separated block copolymer mesophase. In response to the concomitant molecular stretching and collective deformation of the morphology, the system relaxes toward a long-lived, pseudometastable state with a minuscule residual shear stress. Using molecular simulations and self-consistent field theory (SCFT) calculations, we systematically explore the variety of ordered, anisotropic mesostructures that have potential applications in engineering functional materials and can be fabricated by this versatile processing strategy. We study three classes of anisotropic ordered mesostructures, including cylindroids, gyroid-like networks, and sloping lamellae, and show that their domain shape and domain orientation can be independently controlled by the magnitude of the step-shear strain, γ, and the composition of the block copolymer as well as by the way in which we implement the step-shear deformation. We also demonstrate that ..." @default.
- W2897428253 created "2018-10-26" @default.
- W2897428253 creator A5012585792 @default.
- W2897428253 creator A5032918016 @default.
- W2897428253 date "2018-10-16" @default.
- W2897428253 modified "2023-10-12" @default.
- W2897428253 title "Step-Shear Deformation of Block Copolymers" @default.
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- W2897428253 doi "https://doi.org/10.1021/acs.macromol.8b01242" @default.
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