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- W2897439460 abstract "The microwave-assisted catalytic pyrolysis (MACP) of cellulose was carried out using modified HZSM-5 catalysts for bio-oil production. The catalysts of Fe/HZSM-5, Ni/HZSM-5 and Fe–Ni/HZSM-5 were developed and characterized by the X-ray diffraction (XRD) and field-emission scanning electron microscopy (FE-SEM). The bio-oil was characterized by the Fourier transform infrared analyzer (FTIR) and gas chromatography/mass spectrometry (GC/MS). Results showed that Fe/HZSM-5 enhanced the yields of bio-oil by 11.4% and decreased the coke by about 24% compared to HZSM-5 without modification. The saccharides in bio-oil disappeared and were totally converted into phenols and low molecular compounds with the catalysis of Fe–Ni/HZSM-5. Fe–Ni/HZSM-5 showed high selectivity of phenols (20.86%) in the bio-oil. It was a unique finding because usually phenols can only be obtained by the pyrolysis of lignin, not cellulose. The formation of phenols from MACP of cellulose was probably caused by the conversion of furans to aromatics in the pores of HZSM-5, and followed by further conversion of aromatics into phenols on the external surface of HZSM-5." @default.
- W2897439460 created "2018-10-26" @default.
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- W2897439460 date "2019-12-01" @default.
- W2897439460 modified "2023-10-14" @default.
- W2897439460 title "Microwave-assisted catalytic pyrolysis of cellulose for phenol-rich bio-oil production" @default.
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- W2897439460 doi "https://doi.org/10.1016/j.joei.2018.10.012" @default.
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