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- W2897481303 abstract "Al coordinates in ZSM-5 showed significant effects on hierarchical structure and T atoms redistribution during NaOH/TPAOH treatment and different catalytic performances in the methanol-to-propylene reaction. NaOH treatment of parent ZSM-5 with a few extra-framework Al sites mainly involved the desilication process, while an additional alumination process was observed when some Al3+ was added into the NaOH solution, which resulted in mesoporous crystals with intact outer shells. Dealumination–realumination and desilication processes occurred with ZSM-5 with distorted four-coordinate, five-coordinate, or six-coordinate Al sites. For TPAOH treatment, the desilication–recrystallization process occurred with parent ZSM-5 and resulted in hollow crystals with ultrasilica shells via Si redistribution, consequently 2.5 times the lifetime of parent ZSM-5 by restricting external coke deposition. By comparison, desilication, dealumination, and (Si, Al)-recystallization were observed for ZSM-5 with distorted four-coor..." @default.
- W2897481303 created "2018-10-26" @default.
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- W2897481303 date "2018-11-02" @default.
- W2897481303 modified "2023-09-27" @default.
- W2897481303 title "Influence of Al Coordinates on Hierarchical Structure and T Atoms Redistribution during Base Leaching of ZSM-5" @default.
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- W2897481303 doi "https://doi.org/10.1021/acs.iecr.8b03539" @default.
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