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- W2897561552 abstract "Abstract A flexible, enantioselective route to highly functionalized α,β-unsaturated δ-lactones has been applied to the synthesis of 7-aza-phomopsolide E and its C-4 epimer. This approach relies on the application of the Noyori asymmetric hydrogenation of furyl ketone to produce the secondary furyl alcohol in high enantioexcess, which can be stereoselectively transformed into α,β-unsaturated-δ-lactones by a short, highly diastereoselective oxidation and reduction sequence. DCC and acid chloride couplings were used to introduce the side chains of the two natural product analogues." @default.
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- W2897561552 date "2018-12-01" @default.
- W2897561552 modified "2023-09-27" @default.
- W2897561552 title "Asymmetric synthesis of 7-aza-phomopsolide E and its C-4 epimer" @default.
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- W2897561552 doi "https://doi.org/10.1016/j.tet.2018.10.036" @default.
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