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- W2897572671 endingPage "15538" @default.
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- W2897572671 abstract "RhIII - and IrIII -catalyzed asymmetric C-H functionalization reactions of arenes have relied on the employment of chiral RhIII /IrIII cyclopentadienyl catalysts, the introduction of chiral carboxylic acids to achiral Cp*RhX2 catalysts, and the integration of both strategies. Despite considerable progress, each reaction only provided a specific configuration of the enantioenriched product when using a particular chiral catalyst. Reported in this work is the enantiodivergent coupling of sulfoximines with various diazo compounds by RhIII -catalyzed desymmetrizing annulation. The enantiodivergence was enabled by a judicious choice of achiral carboxylic acids, and the enantioselectivity correlates with the steric bias of the carboxylic acid and the sulfoximine." @default.
- W2897572671 created "2018-10-26" @default.
- W2897572671 creator A5000959925 @default.
- W2897572671 creator A5061667297 @default.
- W2897572671 creator A5077190285 @default.
- W2897572671 date "2018-10-30" @default.
- W2897572671 modified "2023-10-14" @default.
- W2897572671 title "Enantiodivergent Desymmetrization in the Rhodium(III)‐Catalyzed Annulation of Sulfoximines with Diazo Compounds" @default.
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- W2897572671 doi "https://doi.org/10.1002/anie.201810472" @default.
- W2897572671 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30307097" @default.
- W2897572671 hasPublicationYear "2018" @default.
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