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- W2897574808 abstract "Abstract The design of highly stable, selective and efficient electrocatalysts for CO 2 reduction reaction is desirable while largely unmet. In this work, a series of precisely designed polyoxometalate-metalloporphyrin organic frameworks are developed. Noted that the integration of {ε-PMo 8 V Mo 4 VI O 40 Zn 4 } cluster and metalloporphyrin endows these polyoxometalate-metalloporphyrin organic frameworks greatly advantages in terms of electron collecting and donating, electron migration and electrocatalytic active component in the CO 2 reduction reaction. Thus-obtained catalysts finally present excellent performances and the mechanisms of catalysis processes are discussed and revealed by density functional theory calculations. Most importantly, Co-PMOF exhibits remarkable faradaic efficiency ( > 94%) over a wide potential range (−0.8 to −1.0 V). Its best faradaic efficiency can reach up to 99% (highest in reported metal-organic frameworks) and it exhibits a high turnover frequency of 1656 h −1 and excellent catalysis stability ( > 36 h)." @default.
- W2897574808 created "2018-10-26" @default.
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- W2897574808 date "2018-10-26" @default.
- W2897574808 modified "2023-10-17" @default.
- W2897574808 title "Oriented electron transmission in polyoxometalate-metalloporphyrin organic framework for highly selective electroreduction of CO2" @default.
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- W2897574808 doi "https://doi.org/10.1038/s41467-018-06938-z" @default.
- W2897574808 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/6203756" @default.
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- W2897574808 hasPublicationYear "2018" @default.
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