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• W2897633508 abstract "The polarization of $mathrm{PbZ}{mathrm{r}}_{0.52}mathrm{T}{mathrm{i}}_{0.48}{mathrm{O}}_{3}$ thin film is switched by changing film thickness through the competition between the strain relaxation-induced flexoelectric fields and the interfacial effects. Without an applied electric field, this reversal of polarization is exploited to control the magnetic properties of $mathrm{L}{mathrm{a}}_{0.67}mathrm{S}{mathrm{r}}_{0.33}mathrm{Mn}{mathrm{O}}_{3}$ by the competition/cooperation between the charge-mediated and the strain-mediated effects. Scanning transmission electron microscopy, polarized near-edge x-ray absorption spectroscopy, and half-integer diffraction measurements are employed to decode the intrinsic magnetoelectric effects in the $mathrm{L}{mathrm{a}}_{0.67}mathrm{S}{mathrm{r}}_{0.33}mathrm{Mn}{mathrm{O}}_{3}/mathrm{PbZ}{mathrm{r}}_{0.52}mathrm{T}{mathrm{i}}_{0.48}{mathrm{O}}_{3}$ heterostructures. With $mathrm{PbZ}{mathrm{r}}_{0.52}mathrm{T}{mathrm{i}}_{0.48}{mathrm{O}}_{3}$ films $<48phantom{rule{0.16em}{0ex}}mathrm{nm}$, the polarization-driven carrier density modulation around the $mathrm{L}{mathrm{a}}_{0.67}mathrm{S}{mathrm{r}}_{0.33}mathrm{Mn}{mathrm{O}}_{3}/mathrm{PbZ}{mathrm{r}}_{0.52}mathrm{T}{mathrm{i}}_{0.48}{mathrm{O}}_{3}$ interface and the strain-mediated Mn $3d$ orbital occupancy work together to enhance the magnetism of 14-unit-cell $mathrm{L}{mathrm{a}}_{0.67}mathrm{S}{mathrm{r}}_{0.33}mathrm{Mn}{mathrm{O}}_{3}$ film; with $mathrm{PbZ}{mathrm{r}}_{0.52}mathrm{T}{mathrm{i}}_{0.48}{mathrm{O}}_{3}$ layers $>48phantom{rule{0.16em}{0ex}}mathrm{nm}$, the strain-induced change of bond length/angle of $mathrm{Mn}{mathrm{O}}_{6}$ accompanied with a modified spin configuration are responsible for the decrease in the Curie temperature and magnetization of 14-unit-cell $mathrm{L}{mathrm{a}}_{0.67}mathrm{S}{mathrm{r}}_{0.33}mathrm{Mn}{mathrm{O}}_{3}$ film." @default.
• W2897633508 created "2018-10-26" @default.
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• W2897633508 date "2019-09-03" @default.
• W2897633508 modified "2023-10-18" @default.
• W2897633508 title "Thickness-dependent polarization-induced intrinsic magnetoelectric effects in <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:mrow><mml:mi mathvariant=normal>L</mml:mi><mml:msub><mml:mi mathvariant=normal>a</mml:mi><mml:mrow><mml:mn>0.67</mml:mn></mml:mrow></mml:msub><mml:mi mathvariant=normal>S</mml:mi><mml:msub><mml:mi mathvariant=normal>r</mml:mi><mml:mrow><mml:mn>0.33</mml:mn></mml:mrow></mml:msub><mml:mi>Mn</mml:mi><mml:msub><mml:mi mathvariant=normal>O</mml:mi><mml…" @default.
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• W2897633508 doi "https://doi.org/10.1103/physrevb.100.104405" @default.
• W2897633508 hasPublicationYear "2019" @default.
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