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• W2897738890 abstract "Abstract Silver‐based electrocatalysts are active in catalyzing electrochemical reduction of CO 2 to CO. We herein report synthesis of capping ligand‐free Ag cubes and octahedra by morphology‐preserved CO reduction from corresponding Ag 2 O counterparts and their performance in electrochemical reduction of CO 2 . Ag cubes are much more active than Ag octahedra and exhibit a stable CO formation rate as high as 142.4 mmol CO g cat −1 h −1 at −0.95 V (vs. RHE). Ag films transiently formed on Ag 2 O crystals during CO 2 electroreduction were observed more active than Ag crystals, revealing a promoting effect of Ag 2 O substrate on electrocatalytic activity of Ag film. These results clearly identify a facet sensitivity of silver electrocatalysts and highlight the importance of surface cleanness of Ag colloids as efficient electrocatalysts." @default.
• W2897738890 created "2018-10-26" @default.
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• W2897738890 date "2018-10-24" @default.
• W2897738890 modified "2023-10-18" @default.
• W2897738890 title "Facet Sensitivity of Capping Ligand‐Free Ag Crystals in CO₂ Electrochemical Reduction to CO" @default.
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• W2897738890 doi "https://doi.org/10.1002/cctc.201801423" @default.
• W2897738890 hasPublicationYear "2018" @default.
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