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- W2897800612 abstract "The formation of hydrogen overlayers on the Zn-terminated $mathrm{ZnO}(0001)$ surface has been reexamined by angle-resolved photoemission spectroscopy (ARPES). While low-energy electron diffraction patterns display the same (1 ifmmodetimeselsetexttimesfi{} 1) symmetry for different surface preparations, the electronic structure feature close to the Fermi level shows the formation of electron pockets, compatible with hydrogen-induced metallic states. Using ARPES and density functional theory (DFT) calculations, we show that hydrogen adspecies can also lead to metallization of this zinc-oxide surface in a similar manner as observed previously on $mathrm{ZnO}(10overline{1}0)$ and O-terminated $mathrm{ZnO}(000overline{1})$. Importantly, our DFT calculations indicate that these electron pockets are formed by $sp$ hybridized states and therefore the angular distribution of the emitted photoelectron is significantly suppressed at the normal emission." @default.
- W2897800612 created "2018-10-26" @default.
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- W2897800612 date "2018-10-15" @default.
- W2897800612 modified "2023-09-23" @default.
- W2897800612 title "Hydrogen-induced metallization on the ZnO(0001) surface" @default.
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- W2897800612 doi "https://doi.org/10.1103/physrevb.98.155416" @default.
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