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- W2897844169 abstract "Nitrogen doped carbon materials have been found to be a capable oxygen electrocatalyst for low-cost and highly durable metal-oxygen batteries. However, it is still a challenge to associate the precise working mechanism with their molecular structure, specific surface area and conductivity. By using first-principles calculations and experimental studies, for the first time, we clarify the higher catalyst activity of pyridinic-N than graphitic-N in highly conductive and porous carbon framework. Accordingly, an ultrahigh conductive three-dimensional doped carbon framework that consists of networked and hollow pipelines with nanometer-thick walls is prepared. Benefiting from such a unique structure, the as-made carbon framework as binder-free cathode for hybrid Li-O2 battery delivers 150 cycles at 1 A g−1 on deep (dis)charge. More importantly, based on the total mass of pyridinic nitrogen doped carbon framework, the capacity of the Li-O2 battery containing the binder-free carbon framework cathode amounts to 49.5 Ah g−1." @default.
- W2897844169 created "2018-10-26" @default.
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- W2897844169 date "2019-02-01" @default.
- W2897844169 modified "2023-09-23" @default.
- W2897844169 title "Highly conductive doped carbon framework as binder-free cathode for hybrid Li-O2 battery" @default.
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- W2897844169 doi "https://doi.org/10.1016/j.carbon.2018.10.045" @default.
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