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• W2897870939 endingPage "13413" @default.
• W2897870939 startingPage "13402" @default.
• W2897870939 abstract "A novel cobalt-catalyzed C-H alkylation of arenes and olefins is achieved with (pyridin-2-yl)isopropyl amine as an N, N-bidentate directing group. Different linear, branched, and cyclic alkyl ethers were used as practical secondary alkylating reagents through cleavage of C(sp3)-O bond, providing an efficient approach to the synthesis of verstile o-alkylated arylamides and tetrasubstituted acrylamides. Mechanistic studies indicate that cleavage of the inert C(sp3)-O bond involves a cobalt-promoted radical process and that cleavage of the inert C(sp2)-H bond by a cobalt catalyst is a rate-limiting step." @default.
• W2897870939 created "2018-10-26" @default.
• W2897870939 creator A5046170578 @default.
• W2897870939 creator A5054315282 @default.
• W2897870939 creator A5066887020 @default.
• W2897870939 creator A5078422118 @default.
• W2897870939 date "2018-10-12" @default.
• W2897870939 modified "2023-10-18" @default.
• W2897870939 title "Cobalt-Catalyzed Secondary Alkylation of Arenes and Olefins with Alkyl Ethers through the Cleavage of C(sp²)–H and C(sp³)–O Bonds" @default.
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• W2897870939 doi "https://doi.org/10.1021/acs.joc.8b02197" @default.
• W2897870939 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30351937" @default.
• W2897870939 hasPublicationYear "2018" @default.
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