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• W2897878404 abstract "Abstract A 3-D inorganic-organic network based on kiggen-type arsenotungstat, [Ag(4,4′-bpy)]2[{Ag(4,4′-bpy)}2(AsWVI11WVO40)]·3H2O(1) (4,4′-bpy = 4,4′-bipyridine), has been synthesized by hydrothermal means. X-ray single crystal analysis shows that compound 1 contains two crystallography independent silver ions, which adopt different coordination modes connecting bpy ligand alternately to form two kinds of metal-organic chains {Agbpy}n. Two parallel {Ag(1)bpy}n chains are linked together via {AsW12O40} linkers to result in a unique sandwich-type dimer chain along a axis. Each Keggin cluster on sandwich chain bonds with six cognate clusters on six adjacent sandwich chains via surrounding six Ag, forming a 2-D layer along c axis. The 2D layer and 1D sandwich chains are intersected to yield a 3D network with 1-D channel. The {Ag(2)bpy}n chains and lattice water reside in the channel and further stabilize the 3-D framework via H-bonding and π-π accumulation. From topological perspective, compound 1 can be viewed as a 3, 6-connected network with {43}2{46.66.83} topology. Compound 1 shows merit electrocatalytic activity for reduction of H2O2 and efficient catalytic degradation ability for three typical dyes under UV radiation." @default.
• W2897878404 created "2018-10-26" @default.
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• W2897878404 date "2018-12-01" @default.
• W2897878404 modified "2023-10-15" @default.
• W2897878404 title "A 3,6-connected 3-D arsenotungstate framework based on unique sandwich-type metal-organic dimer chain" @default.
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• W2897878404 doi "https://doi.org/10.1016/j.inoche.2018.10.005" @default.
• W2897878404 hasPublicationYear "2018" @default.
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