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- W2897976441 abstract "Herein, we report that highly dispersed copper–cobalt mixed metal/metal oxide nanoparticles embedded into three-dimensional porous carbon were highly catalytic active nanocomposites for transforming bioderived furfural (FAL) to cyclopentanone (CPO) via aqueous-phase hydrogenation/rearrangement. This simple and efficient catalyst was prepared by controlled pyrolysis procedure using glucose as the carbon source at 500 °C under N2 atmosphere. Characterization of the as-prepared CuCo0.8@C-500 catalyst by XRD, STEM, SEM, TEM, and XPS suggested that there was a synergism between copper and cobalt. Under an extremely low H2 pressure (0.5 MPa), 90.2% yield of CPO could be attained at 150 °C. In addition, the sample could be recycled for several times without decrease in catalytic activity. Two critical reaction intermediates of furfuryl alcohol (FOL) and 2-cyclopentenone (2-CPE) were detected in the tandem catalytic process. These results demonstrated that this synthetic strategy represented a simple and effective way for utilization of inexpensive biomass resources to obtain some valuable chemicals." @default.
- W2897976441 created "2018-10-26" @default.
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- W2897976441 date "2018-10-09" @default.
- W2897976441 modified "2023-10-14" @default.
- W2897976441 title "In Situ Synthesis of Highly Dispersed Cu–Co Bimetallic Nanoparticles for Tandem Hydrogenation/Rearrangement of Bioderived Furfural in Aqueous-Phase" @default.
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- W2897976441 doi "https://doi.org/10.1021/acssuschemeng.8b03418" @default.
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