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• W2898013695 abstract "The nature of H-atoms adsorbed on M0 -nanoparticles is of major importance in many catalyzed reduction processes. Using isotope labeling, we determined that hydrogen evolution from transient {(M0 -NP)-Hn }n- proceeds mainly via the Heyrovsky mechanism when n is large (i.e., the hydrogens behave as hydrides) but mainly via the Tafel mechanism when n is small (i.e., the hydrogens behave as atoms). Additionally, the relative contributions of the two mechanisms differ considerably for M=Au and Ag. The results are analogous to those recently reported for the M0 -NP-catalyzed de-halogenation processes." @default.
• W2898013695 created "2018-10-26" @default.
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• W2898013695 date "2018-11-15" @default.
• W2898013695 modified "2023-10-03" @default.
• W2898013695 title "The Chemical Properties of Hydrogen Atoms Adsorbed on M⁰ -Nanoparticles Suspended in Aqueous Solutions: The Case of Ag⁰ -NPs and Au⁰ -NPs Reduced by BD₄ ⁻" @default.
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• W2898013695 doi "https://doi.org/10.1002/anie.201809302" @default.
• W2898013695 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30320944" @default.
• W2898013695 hasPublicationYear "2018" @default.
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