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- W2898073757 abstract "Cellulose nanocrystals have been proved to be ideal reinforcing fillers for rubber. However, the increase in tensile strength always accompanies a reduction in extensibility. In this paper, epoxidized natural rubber (ENR) nanocomposites with dual cross-linking networks by incorporating tunicate cellulose nanocrystals (t-CNs) were prepared. Carboxyl groups were introduced onto t-CNs surface via grafting reaction with maleic anhydride (MAH). Interfacial chemical reaction between carboxyl groups on modified t-CNs and epoxy groups on ENR chains led to formation of covalent cross-linking network. Hydrogen bonds between hydroxyl groups on t-CNs and epoxy groups on ENR chains served as physical cross-linking network. Therefore, uniform dispersion and improved interfacial adhesion were achieved. Meanwhile, the covalent cross-linking network could provide strength and elasticity, while the reversible physical cross-linking network could serve as sacrificing element during stretching and dissipate energy. Therefore, dual cross-linked nanocomposites showed improved strength, modulus, extensibility, and decreased hysteresis compared with sole cross-linked nanocomposites." @default.
- W2898073757 created "2018-10-26" @default.
- W2898073757 creator A5025668318 @default.
- W2898073757 creator A5029739553 @default.
- W2898073757 creator A5040252972 @default.
- W2898073757 date "2018-10-11" @default.
- W2898073757 modified "2023-10-14" @default.
- W2898073757 title "Dual Cross-linked Epoxidized Natural Rubber Reinforced by Tunicate Cellulose Nanocrystals with Improved Strength and Extensibility" @default.
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- W2898073757 doi "https://doi.org/10.1021/acssuschemeng.8b03331" @default.
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