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• W2898338214 startingPage "1803972" @default.
• W2898338214 abstract "Graphitic carbon nitride nanosheet (i.e., g-C3N4) is identified as a suitable graphene analogue due to its high theoretical capacity, wider and vacant structure, and easy synthesis method. Currently, g-C3N4 nanosheet has limited application in lithium-ion batteries (LIBs) which is mainly due to the lack of effective intercalation/deintercalation reaction sites, the high binding energy of the Li to the nanosheet, and insufficient conductivity and stability. Density functional theory calculation predicts that the edges of g-C3N4 fibre have a suitable adsorption energy and bestow a balanced adsorption force and desorption freedom to Li. In order to verify this prediction, g-C3N4 nanofibre is synthesized with the edges and pores, as well as higher pyridinic nitrogen content, using a simple polymerization/polycondensation method. The as-prepared g-C3N4 fibre delivers a remarkable specific capacity of 181.7 mAh g−1, as well as extraordinary stability and power density. At a high rate of 10C, the g-C3N4 fibre still has a specific capacity of 138.6 mAh g−1 even after 5000 cycles, being the best-performing g-C3N4 electrode so far in literature. This work is exemplary in combining theoretical computing and experimental techniques in designing the next generation of electroactive materials for LIBs." @default.
• W2898338214 created "2018-11-02" @default.
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• W2898338214 date "2018-10-16" @default.
• W2898338214 modified "2023-10-10" @default.
• W2898338214 title "Carbon Nitride Nanofibres with Exceptional Lithium Storage Capacity: From Theoretical Prediction to Experimental Implementation" @default.
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• W2898338214 doi "https://doi.org/10.1002/adfm.201803972" @default.
• W2898338214 hasPublicationYear "2018" @default.
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