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- W2898888957 abstract "Increasing level of CO2 in the atmosphere is a serious concern. Converting CO2 waste to a potentially clean fuel methanol, by catalytic hydrogenation, will be highly demanding in the perspective of economy and sustainability. Traditionally, it is produced from syngas at high temperature and pressure by utilizing catalyst (Cu/ZnO/Al2O3). For methanol synthesis, cheap CO2 sources are available at industrial scale through CCS technology but options for low-cost hydrogen are limited. Despite it Cu nanoparticles in the catalyst are initially discrete and well dispersed but slowly they aggregate and separate out from the ZnOx interface diminishing the catalytic activity over time ascribed to less number of active sites. To maintain high catalytic activity and selectivity of this catalyst, its stabilization is very crucial. This problem can be resolved by metal–organic frameworks (MOFs) consisting of pores which anchor Cu/ZnOx nanoparticles in their channels preventing their aggregation as well as their phase separation between Cu and ZnOx interface. Due to strong metal-supported interactions and confinement effects within the MOF lead to more dispersed and ultrasmall nanoparticles for CO2 hydrogenation." @default.
- W2898888957 created "2018-11-09" @default.
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- W2898888957 date "2018-10-31" @default.
- W2898888957 modified "2023-09-26" @default.
- W2898888957 title "Methanol Synthesis from CO2 Hydrogenation Using Metal–Organic Frameworks" @default.
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