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• W2899221451 abstract "Abstract. The thermal equilibrium constant between the chlorine monoxide radical (ClO) and its dimer, chlorine peroxide (ClOOCl), was determined as a function of temperature between 228 and 301 K in a discharge flow apparatus using broadband UV absorption spectroscopy. A third-law fit of the equilibrium values determined from the experimental data provides the expression Keq=2.16×10-27e8527±35K/T cm3 molecule−1 (1σ uncertainty). A second-law analysis of the data is in good agreement. From the slope of the van't Hoff plot in the third-law analysis, the enthalpy of formation for ClOOCl is calculated, ΔHf∘(298K)=130.0±0.6 kJ mol−1. The equilibrium constant results from this study suggest that the uncertainties in Keq recommended in the most recent (year 2015) NASA JPL Data Evaluation can be significantly reduced." @default.
• W2899221451 created "2018-11-09" @default.
• W2899221451 creator A5074307124 @default.
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• W2899221451 date "2019-05-10" @default.
• W2899221451 modified "2023-10-17" @default.
• W2899221451 title "UV spectroscopic determination of the chlorine monoxide (ClO) ∕ chlorine peroxide (ClOOCl) thermal equilibrium constant" @default.
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• W2899221451 doi "https://doi.org/10.5194/acp-19-6205-2019" @default.
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