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- W2899385951 abstract "A Zn(II)-based metal–organic framework [Zn3(TCA)2(DPE)]·DMF·6H2O (referred to as BUT-161) has been solvothermally synthesized by the reaction of a tritopic carboxylic acid 4,4′,4″-nitrilotribenzoic acid (H3TCA), an ancillary ditopic pyridine ligand 1,2-di(4-pyridyl)ethylene (DPE) and Zn(NO3)2·6H2O. The framework of BUT-161 shows a pillar-layered structure, where two-dimensional (2D) layers constructed from trimeric Zn3(–CO2)6 clusters and TCA3− ligands are topologically (3,6)-connected net, and the layers are further pillared by the DPE linkers. The resulting 3D framework contains 1D channels along the b axis. Powder X-ray diffraction (PXRD) patterns and gas adsorption studies reveal that the activated phase of BUT-161, as BUT-161a has permanent porosity with a Brunauer-Emmett-Teller (BET) specific surface area of 308 m2 g−1, although the framework structure shrinks (structure transformation) after guest removal. In addition, it has been found that BUT-161a can selectively adsorb CO2 over N2 or CH4." @default.
- W2899385951 created "2018-11-09" @default.
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- W2899385951 date "2019-01-01" @default.
- W2899385951 modified "2023-10-17" @default.
- W2899385951 title "A Zn(II)-based pillar-layered metal–organic framework: Synthesis, structure, and CO2 selective adsorption" @default.
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- W2899385951 doi "https://doi.org/10.1016/j.poly.2018.10.067" @default.
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