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• W2899581127 abstract "We integrated field measurements, hydroponic experiments, microscopy, and spectroscopy to investigate the effect of Ca(II) on dissolved U(VI) uptake by plants in 1 mM HCO3- solutions at circumneutral pH. The accumulation of U in plants (3.1-21.3 mg kg-1) from the stream bank of the Rio Paguate, Jackpile Mine, New Mexico served as a motivation for this study. Brassica juncea was the model plant used for the laboratory experiments conducted over a range of U (30-700 μg L-1) and Ca (0-240 mg L-1) concentrations. The initial U uptake followed pseudo-second-order kinetics. The initial U uptake rate ( V0) ranged from 4.4 to 62 μg g-1 h-1 in experiments with no added Ca and from 0.73 to 2.07 μg g-1 h-1 in experiments with 12 mg L-1 Ca. No measurable U uptake over time was detected for experiments with 240 mg L-1 Ca. Ternary Ca-U-CO3 complexes may affect the decrease in U bioavailability observed in this study. Elemental X-ray mapping using scanning transmission electron microscopy-energy-dispersive spectrometry detected U-P-bearing precipitates within root cell walls in water free of Ca. These results suggest that root interactions with Ca and carbonate in solution affect the bioavailability of U in plants. This study contributes relevant information to applications related to U transport and remediation of contaminated sites." @default.
• W2899581127 created "2018-11-16" @default.
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• W2899581127 date "2018-11-09" @default.
• W2899581127 modified "2023-10-16" @default.
• W2899581127 title "Effect of Calcium on the Bioavailability of Dissolved Uranium(VI) in Plant Roots under Circumneutral pH" @default.
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• W2899581127 doi "https://doi.org/10.1021/acs.est.8b02724" @default.
• W2899581127 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/6341987" @default.
• W2899581127 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30412391" @default.
• W2899581127 hasPublicationYear "2018" @default.
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