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• W2899649218 abstract "Controlling superconducting phase transition on a two-dimensional (2D) material is of great fundamental and technological interest from the viewpoint of making 2D resistance-free electronic circuits. Here, we demonstrate that a 1T-to-2H phase transition can be induced on the topmost monolayer of bulk (<100 nm thick) 1T-TaS2 by thermal annealing. The monolayer 2H-TaS2 on bulk 1T-TaS2 exhibits a superconducting transition temperature (Tc) of 2.1 K, which is significantly enhanced compared to that of bulk 2H-TaS2. Scanning tunneling microscopy measurements reveal a 3 × 3 charge density wave (CDW) in the phase-switched monolayer at 4.5 K. The enhanced Tc is explained by the suppressed 3 × 3 CDW and a charge-transfer doping from the 1T substrate. We further show that the monolayer 2H-TaS2 could be switched back to 1T phase by applying a voltage pulse. The observed surface-limited superconducting phase transition offers a convenient way to prepare robust 2D superconductivity on bulk 1T-TaS2 crystal, thereby bypassing the need to exfoliate monolayer samples." @default.
• W2899649218 created "2018-11-16" @default.
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• W2899649218 date "2018-11-07" @default.
• W2899649218 modified "2023-10-16" @default.
• W2899649218 title "Surface-Limited Superconducting Phase Transition on 1<i>T</i>-TaS₂" @default.
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• W2899649218 doi "https://doi.org/10.1021/acsnano.8b07379" @default.
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