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• W2899682494 abstract "Three photoluminescent isomeric complexes [Cu3(L4)3]2[CuI]2 (labeled as complexes 1, 2, and 3) were prepared from the same bifunctional organic ligand HL4 (3-(4-pyridyl)-5-methyl-1H-pyrazole) and CuI by careful manipulation of the reaction conditions. Planar trinuclear Cu3(L4)3 and CuI/Cu2I2 units are integrated via N–Cu coordination bonds into Cu3Pz3-CunIn systems (Pz = pyrazolate). Complex 1 is a discrete supramolecular aggregate via cooperative π-acid···base (Cu3···I) and Cu···Cu interactions. Complexes 2 and 3 are 2-fold interpenetrated three-dimensional frameworks. The small size of the CunIn (n = 1 or 2) units and structural diversities in such Cu3Pz3-CunIn systems were realized by preinstalling a methyl group on pyrazole at the 5-position of the ligand. The three complexes exhibit subtly different yellow emissions under UV irradiation in their solid states, originating from their respective triplet excited states of the supramolecular coordination luminophores. These results demonstrate that the structural and luminescent diversities of the Cu3Pz3-CunIn-based complexes can be regulated by substituents." @default.
• W2899682494 created "2018-11-16" @default.
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• W2899682494 date "2018-11-09" @default.
• W2899682494 modified "2023-10-16" @default.
• W2899682494 title "Substituent Influence on Structural and Luminescent Diversities of Cu₃(pyrazolate)₃-Cu_<i>n</i>I_<i>n</i> Coordination Supramolecular Isomers" @default.
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• W2899682494 doi "https://doi.org/10.1021/acs.cgd.8b01476" @default.
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