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- W2900212858 abstract "Photocatalytic organic conversions involving a hydrogen transfer (HT) step have attracted much attention, but the efficiency and selectivity under visible light irradiation still needs to be significantly enhanced. Here we have developed a noble metal-free, basic-site engineered bismuth oxybromide [Bi24O31Br10(OH)δ] that can accelerate the photocatalytic HT step in both reduction and oxidation reactions, i.e., nitrobenzene to azo/azoxybenzene, quinones to quinols, thiones to thiols, and alcohols to ketones under visible light irradiation and ambient conditions. Remarkably, quantum efficiencies of 42% and 32% for the nitrobenzene reduction can be reached under 410 and 450 nm irradiation, respectively. The Bi24O31Br10(OH)δ photocatalyst also exhibits excellent performance in up-scaling and stability under visible light and even solar irradiation, revealing economic potential for industrial applications." @default.
- W2900212858 created "2018-11-16" @default.
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- W2900212858 date "2018-11-05" @default.
- W2900212858 modified "2023-10-06" @default.
- W2900212858 title "Efficient Solar-Driven Hydrogen Transfer by Bismuth-Based Photocatalyst with Engineered Basic Sites" @default.
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- W2900212858 doi "https://doi.org/10.1021/jacs.8b09796" @default.
- W2900212858 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30394730" @default.
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