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- W2901107413 abstract "Abstract Herein, an effective and novel strategy has been designed to increase electrochemical reaction active sites in Ni/NiO nanoparticles prepared by optimizing the annealing temperature of nickel-based metal organic framework (Ni-MOF). Note that the incorporation of Ni3+ into the primitive lattice of Ni/NiO nanoparticles will cause a subtle atomic rearrangement, providing a large number of electrochemical reaction active sites. The density functional theory (DFT) simulation results also exhibit that the introduction of Ni3+ significantly lowers the gibbs free energy of atomic hydrogen absorption on the surface of Ni/NiO, benefiting H2 gas evolution. On the basis of the above advantages, the as-synthesized Ni/NiO nanoparticles exhibit excellent performance for supercapacitors (SCs, the areal specific capacitance of 684.4 m F cm−2 at 1 mA cm−2) and Hydrogen evolution reaction (HER, ultralow overpotential of 41 mV at 10 mA cm−2). Significantly, the all-solid-state flexible asymmetric SCs based on Ni/NiO as anode and CNTs-COOH as cathode displays a high energy density of 61.3 W h kg−1 at the power density of 900 W kg−1. This work highlights the crucial role of the lattice distortion of materials for future applications in the sustainable energy storage and conversion." @default.
- W2901107413 created "2018-11-29" @default.
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- W2901107413 date "2019-05-01" @default.
- W2901107413 modified "2023-10-16" @default.
- W2901107413 title "Metal-organic framework derived Ni/NiO micro-particles with subtle lattice distortions for high-performance electrocatalyst and supercapacitor" @default.
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- W2901107413 doi "https://doi.org/10.1016/j.apcatb.2018.11.035" @default.
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