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- W2901416986 abstract "Abstract Oxygen vacancy modulation has emerged as a prevalent strategy to improve the performance of heterogeneous catalysts. By far, the impact of oxygen vacancy rearrangement on the efficiency of Fenton-like reaction remains largely unknown. In this paper, Fe-containing polyoxometalates were coupled with defect-rearranged TiO2 to construct defective Fenton-like photocatalysts. Experimental characterizations revealed that defect rearrangement facilitated the interfacial transfer of electrons from TiO2 to polyoxometalate molecules. Fenton-like photocatalysts with rearranged defects exhibited 5 and 3.5 times higher activity for the synergetic degradation of toxic dye and 5-Sulfosalicylic acid than pristine TiO2. This enhancement was ascribed to the beneficial role of oxygen vacancy modulation for activating oxygen and H2O2 molecules into O2− and OH radicals. Our work provides new opportunities for exploring efficient Fenton-like photocatalysts for environmental remediation." @default.
- W2901416986 created "2018-11-29" @default.
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- W2901416986 date "2019-05-01" @default.
- W2901416986 modified "2023-10-17" @default.
- W2901416986 title "Polyoxometalates/TiO2 Fenton-like photocatalysts with rearranged oxygen vacancies for enhanced synergetic degradation" @default.
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- W2901416986 doi "https://doi.org/10.1016/j.apcatb.2018.11.063" @default.
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