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• W2901567425 endingPage "11833" @default.
• W2901567425 startingPage "11827" @default.
• W2901567425 abstract "This report describes a carboxylate ligand exchange strategy that was used to achieve a Catellani reaction consisting of amination/unactivated aliphatic C–H arylation. Pivalic acid was used as an additive that could effectively promote C–H activation of unactivated alkanes without affecting the key five-membered aryl-norbornene–palladacycle (ANP) intermediate. Importantly, the reaction demonstrates high regioselectivity for the primary carbon. Following ortho-amination, the carboxylic acid was found to coordinate palladium in a bidentate fashion, and the pathway and driving force of carboxylic acid exchange was explored using density functional theory (DFT) calculations." @default.
• W2901567425 created "2018-11-29" @default.
• W2901567425 creator A5022730595 @default.
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• W2901567425 creator A5047548850 @default.
• W2901567425 creator A5052662458 @default.
• W2901567425 creator A5089482025 @default.
• W2901567425 date "2018-11-12" @default.
• W2901567425 modified "2023-10-16" @default.
• W2901567425 title "Carboxylate Ligand-Exchanged Amination/C(<i>sp</i>³)–H Arylation Reaction via Pd/Norbornene Cooperative Catalysis" @default.
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