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• W2901637141 abstract "Abstract Ammonia (NH 3 ) is vital to human beings as an important energy carrier, fertilizer precursor, and fuel, while breakage of the NN bond in nitrogen (N 2 ) is a kinetically complex and energetically challenging multistep reaction. Development of electrocatalysts for efficient NH 3 electrosynthesis via the N 2 reduction reaction (NRR) is highly desirable but remains a key challenge. In this work, based on the density functional theory calculations, a novel and effective strategy to boost the nitrogen electroreduction performance of BiVO 4 by tailoring its oxygen vacancies (OVs) is first proposed and demonstrated. Unexpectedly, the noble‐metal‐free BiVO 4 with the highest OVs concentration shows excellent NRR performances, including high NH 3 yield rate (up to 8.60 µg h −1 mg −1 cat. ), high faradaic efficiency (10.04% at −0.5 V vs reversible hydrogen electrode), and good stability (up to 24 h) at ambient conditions, outperforming most reported NRR electrocatalysts under ambient conditions and even some under harsh conditions, which can be attributed to enhanced N 2 adsorption energy and a more favorable active reaction site at the V atom with lower coordination and higher spin‐polarization with a localized magnetic moment due to the introduction of OVs." @default.
• W2901637141 created "2018-11-29" @default.
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• W2901637141 date "2018-11-15" @default.
• W2901637141 modified "2023-10-15" @default.
• W2901637141 title "Tailoring Oxygen Vacancies of BiVO₄ toward Highly Efficient Noble‐Metal‐Free Electrocatalyst for Artificial N₂ Fixation under Ambient Conditions" @default.
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• W2901637141 doi "https://doi.org/10.1002/smtd.201800333" @default.
• W2901637141 hasPublicationYear "2018" @default.
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