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• W2901736119 startingPage "152" @default.
• W2901736119 abstract "A new model of the chemical evolution of primordial species in the Recombination Era, focusing on rovibrational molecular level populations and line emission, the main cooling process for low-temperature primordial gas, is presented. Since molecular excitation calculations are vital in determining particle velocity distributions, internal state distributions, abundances, and ionization balance in gaseous environments, our model of the early universe considers nonthermal level populations using new state-to-state collisional excitation rate coefficients and reaction rates. This model of Recombination Era astrochemistry highlights the level populations of , HD, and H2 and expands upon the current chemical networks by considering deuterated, ionized, and excited species. We furthermore couple the heat equation to the chemical network to form a complete model of thermal balance and dynamical evolution of primordial gas in the early universe. A developmental version of the spectral synthesis package Cloudy was used to model the primordial gas, and a data set of vibrational excitation rate coefficients due to H collisions are provided." @default.
• W2901736119 created "2018-11-29" @default.
• W2901736119 creator A5030022439 @default.
• W2901736119 creator A5044693409 @default.
• W2901736119 creator A5065742191 @default.
• W2901736119 date "2018-11-12" @default.
• W2901736119 modified "2023-09-25" @default.
• W2901736119 title "Rovibrational Chemistry of ${{rm{H}}}_{2}^{+}$, HD, and H₂ in the Recombination Era" @default.
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• W2901736119 doi "https://doi.org/10.3847/1538-4357/aae4e3" @default.
• W2901736119 hasPublicationYear "2018" @default.
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