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• W2902004424 startingPage "18074" @default.
• W2902004424 abstract "Providing a mechanically stable and electronically efficient coupling between a molecule and an electrode is critical to the study of charge transfer and conductance of the molecule. A common method is to link the molecule to Au electrodes via a linker (e.g., thiol terminal of the molecule). Here we study the mechanical stability and electronic coupling of a S-Au bond in single-molecule junctions over a broad range of electrode potentials. Our results show that the mechanical and electromechanical properties of molecule-electrode contact undergo a systematic change with the potential involving Au oxidation at positive potentials and S protonation at negative potentials. The study establishes the potential range for a stable S-Au bond and determines the potential dependence of the mechanical and electromechanical properties of the molecule-electrode contact, which is crucial to the interpretation of potential-dependent charge transfer in electrochemistry and electrochemical gating of charge transport in molecular electronics." @default.
• W2902004424 created "2018-12-11" @default.
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• W2902004424 date "2018-11-30" @default.
• W2902004424 modified "2023-10-17" @default.
• W2902004424 title "Potential Dependence of Mechanical Stability and Electronic Coupling of Single S–Au Bonds" @default.
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• W2902004424 doi "https://doi.org/10.1021/jacs.8b10857" @default.
• W2902004424 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30500187" @default.
• W2902004424 hasPublicationYear "2018" @default.
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