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- W2902273624 abstract "An organic-inorganic hybrid coating with spatial structures is known to be potential for biology, catalysis, and electrochemistry, but no report of basket-weave structure made from organic component has been available. Here, we report a molecular self-assembly to create the basket-weave organic structure using dimethyl-5-hydroxyisophthalate (DMIP). Primary clusters of DMIP precipitated on the porous surface of inorganic layer by the use of beneficial effect of the micro-defects which triggers the physical locking activated by charge-transfer phenomena. Then, the organic chain grows on a certain plane, resulting from the non-covalent π-π stackings between short-range ordered aromatic cores as well as the interactions between polar functional groups. A detailed analysis on surface morphologies suggests that two adjacent basket-weaves are linked together through kinds of non-covalent interactions between functional groups of each weave. Thus, the molecule agglomerates of basket-weave organic component formed on defective inorganic layer are the primary source for extraordinary electrochemical stability." @default.
- W2902273624 created "2018-12-11" @default.
- W2902273624 creator A5046595967 @default.
- W2902273624 creator A5080169938 @default.
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- W2902273624 date "2019-03-01" @default.
- W2902273624 modified "2023-09-27" @default.
- W2902273624 title "Self-assembly of basket-weave organic layer formed on defective inorganic surface" @default.
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- W2902273624 doi "https://doi.org/10.1016/j.cej.2018.11.221" @default.
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