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- W2902496329 abstract "Efficient removal of phosphate by agricultural waste derived materials from wastewater is an effective and economic way to prevent eutrophication and water bloom. In this work, we proposed a novel method to immobilize a water stable metal organic framework UiO-66 nanoparticle within modified wheat straw through in-situ hydrothermal synthesis and obtained the new UiO-66 nanocomposites. As indicated by SEM and BET analyses, UiO-66 is uniformly dispersed on the surface and the inner pores of modified wheat straws. The utilization rate of active sites is significantly promoted after UiO-66 impregnation within positively charged wheat straw (St+@UiO-66) which is more beneficial for UiO-66 dispersion. The saturated adsorption capacity of hybrid St+@UiO-66 is shown to be more than 2 times greater than bulky one under high ionic strength. Compared to commercial anion exchanger D201, St+@UiO-66 exhibits excellent selectivity and preference toward phosphate. The adsorption process is highly pH-dependent and adsorption kinetics data fitted well with the pseudo-second-order model. FTIR and XPS study indicated that hydroxyl groups on the surface of UiO-66 were replaced by phosphate ions and the inner-sphere complexation was formed via establishing Zr–O–P coordination bonds. In addition, St+@UiO-66 could be sustainably employed for phosphate removal through the combination of periodic regeneration and complete regeneration. It is demonstrated that St+@UiO-66 has preferable adsorption of phosphate with improved utilization of active sites, implying great potential as a promising phosphate adsorbent." @default.
- W2902496329 created "2018-12-11" @default.
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- W2902496329 date "2019-03-01" @default.
- W2902496329 modified "2023-10-16" @default.
- W2902496329 title "Fabrication of agricultural waste supported UiO-66 nanoparticles with high utilization in phosphate removal from water" @default.
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- W2902496329 doi "https://doi.org/10.1016/j.cej.2018.12.017" @default.
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