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• W2902962008 abstract "Abstract Inspired by natural photosynthesis, the design of new Z‐scheme photocatalytic systems is very promising for boosting the photocatalytic performance of H 2 production and CO 2 reduction; however, until now, the direct synthesis of efficient Z‐scheme photocatalysts remains a grand challenge. Herein, it is demonstrated that an interesting Z‐scheme photocatalyst can be constructed by coupling In 2 O 3 and ZnIn 2 Se 4 semiconductors based on theoretical calculations. Experimentally, a class of ultrathin In 2 O 3 –ZnIn 2 Se 4 (denoted as In 2 O 3 –ZISe) spontaneous Z‐scheme nanosheet photocatalysts for greatly enhancing photocatalytic H 2 production is made. Furthermore, Mo atoms are incorporated in the Z‐scheme In 2 O 3 –ZISe nanosheet photocatalyst by forming the MoSe bond, confirmed by X‐ray photoelectron spectroscopy, in which the formed MoSe 2 works as cocatalyst of the Z‐scheme photocatalyst. As a consequence, such a unique structure of In 2 O 3 –ZISe–Mo makes it exhibit 21.7 and 232.6 times higher photocatalytic H 2 evolution activity than those of In 2 O 3 –ZnIn 2 Se 4 and In 2 O 3 nanosheets, respectively. Moreover, In 2 O 3 –ZISe–Mo is also very stable for photocatalytic H 2 production by showing almost no activity decay for 16 h test. Ultraviolet–visible diffuse reflectance spectra, photoluminescence spectroscopy, transient photocurrent spectra, and electrochemical impedance spectroscopy reveal that the enhanced photocatalytic performance of In 2 O 3 –ZISe–Mo is mainly attributed to its widened photoresponse range and effective carrier separation because of its special structure." @default.
• W2902962008 created "2018-12-11" @default.
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• W2902962008 date "2018-12-05" @default.
• W2902962008 modified "2023-10-14" @default.
• W2902962008 title "Ultrathin Visible-Light-Driven Mo Incorporating In₂ O₃ -ZnIn₂ Se₄ Z-Scheme Nanosheet Photocatalysts" @default.
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• W2902962008 doi "https://doi.org/10.1002/adma.201807226" @default.
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