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- W2903617042 abstract "The observation of long-range energy propagation along nano-engineered arrays of bacterial antenna complexes has been recurrently addressed as a result of ballistic, hence, coherent propagation. We show that the experimentally determined quantities relevant for these dynamics hinder the formation of large coherent domains and inevitably lead to classical diffusion in these densely packed arrays, which nevertheless benefit from the spectral complexity of single antenna complexes and near field interactions to result in the propagation observed. We show that the packing density bridges the apparent incompatibility between observed energy transfer rates in bacterial photosynthetic membranes and nano-engineered antenna arrays, which together with exciton delocalization across individual antennas and non-equilibrium transport, provides useful design strategies to optimize energy transfer in the presence of typical room temperature conditions." @default.
- W2903617042 created "2018-12-22" @default.
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- W2903617042 date "2018-12-19" @default.
- W2903617042 modified "2023-09-27" @default.
- W2903617042 title "Non-equilibrium speed-up and dark state shelving tuned by near field exciton transfer in nano-engineered biomimetic arrays" @default.
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