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- W2903855360 abstract "We study the nature of photoexcited charge carriers in ${mathrm{CsPbBr}}_{3}$ nanocrystal thin films by ultrafast optical pump-THz probe spectroscopy. We observe a deviation from a pure Drude dispersion of the THz dielectric response that is ascribed to the polaronic nature of carriers; a transient blueshift of observed phonon frequencies is indicative of the coupling between photogenerated charges and stretching-bending modes of the deformed inorganic sublattice, as confirmed by DFT calculations." @default.
- W2903855360 created "2018-12-22" @default.
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- W2903855360 date "2019-04-24" @default.
- W2903855360 modified "2023-10-15" @default.
- W2903855360 title "Ultrafast THz Probe of Photoinduced Polarons in Lead-Halide Perovskites" @default.
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- W2903855360 doi "https://doi.org/10.1103/physrevlett.122.166601" @default.
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