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- W2903889435 abstract "We show that for a quantum system coupled to both vibrational and electromagnetic environments, enforcing additivity of their combined influences results in nonequilibrium dynamics that does not respect the Franck-Condon principle. We overcome this shortcoming by employing a collective coordinate representation of the vibrational environment, which permits the derivation of a nonadditive master equation. When applied to a two-level emitter our treatment predicts decreasing photon emission rates with increasing vibrational coupling, consistent with Franck-Condon physics. In contrast, the additive approximation predicts the emission rate to be completely insensitive to vibrations. We find that nonadditivity also plays a key role in the stationary nonequilibrium model behavior, enabling two-level population inversion under incoherent electromagnetic excitation." @default.
- W2903889435 created "2018-12-22" @default.
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- W2903889435 date "2019-08-28" @default.
- W2903889435 modified "2023-10-05" @default.
- W2903889435 title "Environmental Nonadditivity and Franck-Condon physics in Nonequilibrium Quantum Systems" @default.
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- W2903889435 doi "https://doi.org/10.1103/physrevlett.123.093601" @default.
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