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• W2904136513 abstract "The hydrogen-deficient and oxygen-rich nature of lignocellulosic biomass prohibits effective conversions of biomass to fuels and chemicals via catalytic pyrolysis due to significant coking of the catalysts. Co-feeding of biomass feedstock with hydrogen-rich and oxygen-deficient thermoplastics could improve the process. Herein, thermal and catalytic co-pyrolysis of cellulose and polyethylene (PE) was studied via thermogravimetry combined with an online photoionization time-of-flight mass spectrometry (PI-TOF-MS). No notable synergetic effect was found in the thermal co-pyrolysis process while a considerable synergetic effect was observed during the catalytic co-pyrolysis. In the case of catalytic pyrolysis, co-feeding of cellulose with PE significantly improved the aromatic formation. Detailed reaction intermediates and products were detected by PI-TOF-MS and the process of aromatization could be ascribed to aromatization of small oxygenates and olefins, as well as Diels-Alder reaction and dehydration by HZSM-5. Moreover, this study provides a reliable tool for screening and optimizing of catalytic co-pyrolysis." @default.
• W2904136513 created "2018-12-22" @default.
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• W2904136513 date "2019-03-01" @default.
• W2904136513 modified "2023-10-14" @default.
• W2904136513 title "Online photoionization mass spectrometric evaluation of catalytic co-pyrolysis of cellulose and polyethylene over HZSM-5" @default.
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• W2904136513 doi "https://doi.org/10.1016/j.biortech.2018.12.045" @default.
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• W2904136513 hasPublicationYear "2019" @default.
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