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• W2904282079 abstract "The continuously increasing number and size of lithium-based batteries developed for large-scale applications raise serious environmental concerns. Herein, we address the issues related to electrolyte toxicity and safety by proposing a water-in-ionomer type of electrolyte which replaces organic solvents by water and expensive and toxic fluorinated lithium salts by a non-fluorinated, inexpensive and non-toxic superabsorbing ionomer, lithium polyacrylate. Interestingly, the electrochemical stability window of this electrolyte is extended greatly, even for high water contents. Particularly, the gel with 50 wt% ionomer exhibits an electrochemical stability window of 2.6 V vs. platinum and a conductivity of 6.5 mS cm-1 at 20 °C. Structural investigations suggest that the electrolytes locally self-organize and most likely switch local structures with the change of water content, leading to a 50% gel with good conductivity and elastic properties. A LiTi2(PO4)3/LiMn2O4 lithium-ion cell incorporating this electrolyte provided an average discharge voltage > 1.5 V and a specific energy of 77 Wh kg-1, while for an alternative cell chemistry, i.e., TiO2/LiMn2O4, a further enhanced average output voltage of 2.1 V and an initial specific energy of 124.2 Wh kg-1 are achieved." @default.
• W2904282079 created "2018-12-22" @default.
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• W2904282079 date "2018-12-14" @default.
• W2904282079 modified "2023-10-17" @default.
• W2904282079 title "Fluorine-free water-in-ionomer electrolytes for sustainable lithium-ion batteries" @default.
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• W2904282079 doi "https://doi.org/10.1038/s41467-018-07331-6" @default.
• W2904282079 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/6294254" @default.
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