Matches in SemOpenAlex for { <https://semopenalex.org/work/W2904295306> ?p ?o ?g. }
- W2904295306 endingPage "973" @default.
- W2904295306 startingPage "969" @default.
- W2904295306 abstract "Abstract Magnetic resonance imaging (MRI) is a powerful technique to characterize reactors during operating catalytic processes. However, MRI studies of heterogeneous catalytic reactions are particularly challenging because the low spin density of reacting and product fluids (for gas phase reactions) as well as magnetic field inhomogeneity, caused by the presence of a solid catalyst inside a reactor, exacerbate already low intrinsic sensitivity of this method. While hyperpolarization techniques such as parahydrogen induced polarization (PHIP) can substantially increase the NMR signal intensity, this general strategy to enable MR imaging of working heterogeneous catalysts to date remains underexplored. Here, we present a new type of model catalytic reactors for MRI that allow the characterization of a heterogeneous hydrogenation reaction aided by the PHIP signal enhancement, but also suitable for the imaging of regular non‐polarized gases. These catalytic systems permit exploring the complex interplay between chemistry and fluid‐dynamics that are typically encountered in practical systems, but mostly absent in simple batch reactors. High stability of the model reactors at catalytic conditions and their fabrication simplicity make this approach compelling for in situ studies of heterogeneous catalytic processes by MRI." @default.
- W2904295306 created "2018-12-22" @default.
- W2904295306 creator A5007422032 @default.
- W2904295306 creator A5012781928 @default.
- W2904295306 creator A5015140879 @default.
- W2904295306 creator A5018689283 @default.
- W2904295306 creator A5022808398 @default.
- W2904295306 creator A5024347042 @default.
- W2904295306 creator A5024554829 @default.
- W2904295306 creator A5038755479 @default.
- W2904295306 creator A5060022719 @default.
- W2904295306 creator A5060459445 @default.
- W2904295306 date "2019-01-09" @default.
- W2904295306 modified "2023-10-17" @default.
- W2904295306 title "Robust In Situ Magnetic Resonance Imaging of Heterogeneous Catalytic Hydrogenation with and without Hyperpolarization" @default.
- W2904295306 cites W150662263 @default.
- W2904295306 cites W194015576 @default.
- W2904295306 cites W1969665854 @default.
- W2904295306 cites W1975585032 @default.
- W2904295306 cites W1976716413 @default.
- W2904295306 cites W1977573245 @default.
- W2904295306 cites W1981392446 @default.
- W2904295306 cites W1982058937 @default.
- W2904295306 cites W1988564310 @default.
- W2904295306 cites W1989167922 @default.
- W2904295306 cites W1993815337 @default.
- W2904295306 cites W1995062034 @default.
- W2904295306 cites W1997172214 @default.
- W2904295306 cites W1998337949 @default.
- W2904295306 cites W2004550766 @default.
- W2904295306 cites W2009364474 @default.
- W2904295306 cites W2011619983 @default.
- W2904295306 cites W2012925774 @default.
- W2904295306 cites W2015147781 @default.
- W2904295306 cites W2017111606 @default.
- W2904295306 cites W2019631503 @default.
- W2904295306 cites W2028326663 @default.
- W2904295306 cites W2034059832 @default.
- W2904295306 cites W2044836101 @default.
- W2904295306 cites W2047904261 @default.
- W2904295306 cites W2052220397 @default.
- W2904295306 cites W2057017828 @default.
- W2904295306 cites W2059249500 @default.
- W2904295306 cites W2059900570 @default.
- W2904295306 cites W2063179381 @default.
- W2904295306 cites W2064054946 @default.
- W2904295306 cites W2067731236 @default.
- W2904295306 cites W2090051635 @default.
- W2904295306 cites W2090899513 @default.
- W2904295306 cites W2091670229 @default.
- W2904295306 cites W2100832144 @default.
- W2904295306 cites W2101363148 @default.
- W2904295306 cites W2102906871 @default.
- W2904295306 cites W2104052148 @default.
- W2904295306 cites W2118334283 @default.
- W2904295306 cites W2128331254 @default.
- W2904295306 cites W2133632784 @default.
- W2904295306 cites W2144116940 @default.
- W2904295306 cites W2157518820 @default.
- W2904295306 cites W2160037375 @default.
- W2904295306 cites W2170534922 @default.
- W2904295306 cites W2276134523 @default.
- W2904295306 cites W2331350789 @default.
- W2904295306 cites W2335551685 @default.
- W2904295306 cites W2477988574 @default.
- W2904295306 cites W2510567329 @default.
- W2904295306 cites W2586323124 @default.
- W2904295306 cites W2605388137 @default.
- W2904295306 cites W2613657217 @default.
- W2904295306 cites W2766032390 @default.
- W2904295306 cites W2783883563 @default.
- W2904295306 cites W2793497834 @default.
- W2904295306 cites W2809190810 @default.
- W2904295306 cites W2883647481 @default.
- W2904295306 cites W2886845821 @default.
- W2904295306 cites W4211220677 @default.
- W2904295306 cites W4231320020 @default.
- W2904295306 cites W4238017914 @default.
- W2904295306 cites W4239979533 @default.
- W2904295306 cites W4248329774 @default.
- W2904295306 cites W4250039025 @default.
- W2904295306 cites W4252880381 @default.
- W2904295306 cites W634953094 @default.
- W2904295306 cites W831292531 @default.
- W2904295306 doi "https://doi.org/10.1002/cctc.201801820" @default.
- W2904295306 hasPublicationYear "2019" @default.
- W2904295306 type Work @default.
- W2904295306 sameAs 2904295306 @default.
- W2904295306 citedByCount "7" @default.
- W2904295306 countsByYear W29042953062019 @default.
- W2904295306 countsByYear W29042953062021 @default.
- W2904295306 countsByYear W29042953062022 @default.
- W2904295306 crossrefType "journal-article" @default.
- W2904295306 hasAuthorship W2904295306A5007422032 @default.
- W2904295306 hasAuthorship W2904295306A5012781928 @default.
- W2904295306 hasAuthorship W2904295306A5015140879 @default.
- W2904295306 hasAuthorship W2904295306A5018689283 @default.
- W2904295306 hasAuthorship W2904295306A5022808398 @default.