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- W2904332468 abstract "The pressure behavior of crystalline Cs2UO2Cl4 has been explored using a diamond anvil cell. The uranyl fluorescence intensity decreases dramatically with increasing pressure. Using the O-U-O symmetric stretching frequency, an apparent linear decrease in bond length with increasing pressure was observed. A linear decrease in fluorescence intensity with increasing pressure was attributed to a large growth in the nonradiative relaxation, likely attributed to increased relaxation through phonon modes. Quantum theory of atoms in molecules calculations and ab initio wave function methods (CASSCF) support the U≡O bond in UO22+ being highly sensitive to the bond distance, but negligibly affected by the U-Cl bond length." @default.
- W2904332468 created "2018-12-22" @default.
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- W2904332468 date "2018-12-20" @default.
- W2904332468 modified "2023-10-18" @default.
- W2904332468 title "High-Pressure Studies of Cesium Uranyl Chloride" @default.
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- W2904332468 doi "https://doi.org/10.1021/acs.inorgchem.8b02300" @default.
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