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- W2904686566 abstract "Abstract Due to cage-like voids in the lattice, skutterudite NiP3 is regarded as a promising negative electrode material with high specific capacity. The fabrication of phosphide based on ceramic routes always leads to multiphase formation and serious agglomeration of particles. The resultant cycle performance is thus to be improved. In this paper, single phase skutterudite NiP3 particles (NNP) were fabricated by the reaction of NiS precursor with red phosphorus. As comparison, skutterudite NiP3 was also prepared by the direct reaction of Ni with red phosphorus (MNP). After 50 cycles, NNP retained 712 mAh g−1 at current density of 159.1 mAg−1, while MNP delivered a capacity less than that of commercial graphite within 16 cycles. According to CV analysis, the improvement in cycling performance of NNP was attributed to an insertion-dominated two-step lithiation process, while MNP undergone a straightforward conversion process. The formation of layer-structured intermediate LixNiP3 phase by an insertion reaction would compete with the direct generation of Li3P and Ni (0) composites by a typical conversion reaction. The improvement in the rating performance originates from the low-impedance of charge transfer and fast migration of Li+ in the electrode of NNP." @default.
- W2904686566 created "2018-12-22" @default.
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- W2904686566 date "2019-04-01" @default.
- W2904686566 modified "2023-10-16" @default.
- W2904686566 title "Size effect on the electrochemical reaction path and performance of nano size phosphorus rich skutterudite nickle phosphide" @default.
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- W2904686566 doi "https://doi.org/10.1016/j.jallcom.2018.12.121" @default.
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