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- W2904805003 abstract "The climatic effect of atmospheric particles is greatly dependent on their hygroscopicity and chemical composition. Although the hygroscopic behavior of individual components of aerosol has been widely studied, the effect of coexisting species on the hygroscopic behavior of mixed constituents is still not clear. In this study, we used Raman spectroscopy to investigate how particles with different hygroscopic behaviors affect each other when they are combined together in mixtures. The effect of coexisting hygroscopic components, e.g. NaCl, NH4NO3, and (NH4)2SO4, on the hygroscopic behavior of externally mixed H2C2O4/CaCO3 was studied. We found that coexisting NH4NO3 can promote the conversion of H2C2O4/CaCO3 to CaC2O4·H2O in the humidifying process by providing a deliquesced solution to dissolve H+ in the oxalic acid matrix. Moreover, competition and blocking effects existed in the case of coexisting (NH4)2SO4. Reactions between (NH4)2SO4 and CaCO3 led to the formation of CaSO4·2H2O and (NH4)2C2O4 instead of CaC2O4. NaCl reacted with H2C2O4 in solution to form Na2C2O4. These results suggested that synergistic effects between coexisting components in mixed particles during the humidifying-dehumidifying process may change their chemical composition, mixing state, and hygroscopicity. In addition, chemical reactions should be considered in future studies on the hygroscopic behavior of mixed particles." @default.
- W2904805003 created "2018-12-22" @default.
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- W2904805003 date "2019-03-01" @default.
- W2904805003 modified "2023-10-17" @default.
- W2904805003 title "A laboratory study on the hygroscopic behavior of H2C2O4-containing mixed particles" @default.
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- W2904805003 doi "https://doi.org/10.1016/j.atmosenv.2018.11.056" @default.
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