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- W2905313447 abstract "A dual or multiple stable isotope relationship, for example, a trajectory in a δ−δ (or δ′−δ′) space, can be used to deduce the relationship of underlying diagnostic isotope fractionation factors (α) and therefore reveal the mechanism of a reaction process. While temporal data sampled from a closed-system can be treated by a Rayleigh distillation model, spatial data should be treated by a reaction-transport model. Owing to an apparent similarity between the temporal and spatial trajectories, the research community has often ignored this distinction and applied a Rayleigh distillation model to cases where a reaction-transport model should be applied. To examine the potential error of this practice, here we compare the results of a Rayleigh distillation model to a diffusional reaction-transport model by simulating the trajectories in nitrate’s δ′18O−δ′15N space during a simple denitrification process. We found that an incorrect application of a Rayleigh distillation model can underestimate the degree of a di..." @default.
- W2905313447 created "2018-12-22" @default.
- W2905313447 creator A5017506877 @default.
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- W2905313447 date "2018-12-06" @default.
- W2905313447 modified "2023-10-16" @default.
- W2905313447 title "Predicting High-Dimensional Isotope Relationships from Diagnostic Fractionation Factors in Systems with Diffusional Mass Transfer" @default.
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- W2905313447 doi "https://doi.org/10.1021/acsearthspacechem.8b00149" @default.
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