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- W2905977872 abstract "Amine/Pd(II) cooperative catalysis has enabled a highly enantioselective addition of cyclic ketones to unactivated alkenes. The hallmark of the strategy includes amide-directed, regioselective activation of alkenes by Pd(II) and enhancing the nucleophilicity of α-carbon of the ketones by enamine catalysis to synergistically drive the reaction, which is basically unable to be accessed by a single catalyst. The combination of a commercially available Pd(II) catalyst and diphenylprolinol was able to provide the γ-addition products with good to high yields and efficient stereochemical control (up to 95% ee)." @default.
- W2905977872 created "2019-01-01" @default.
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- W2905977872 date "2018-12-21" @default.
- W2905977872 modified "2023-09-29" @default.
- W2905977872 title "Enantioselective Addition of Cyclic Ketones to Unactivated Alkenes Enabled by Amine/Pd(II) Cooperative Catalysis" @default.
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- W2905977872 doi "https://doi.org/10.1021/acscatal.8b04654" @default.
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