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• W2907019107 abstract "Abstract Owing to the strong nonpolar bonds involved, selective C−H functionalization of methane and ethane to esters remains a challenge for molecular homogeneous chemistry. We report that the computationally predicted main‐group p ‐block Sb V (TFA) 5 complex selectively functionalizes the C−H bonds of methane and ethane to the corresponding mono and/or diol trifluoroacetate esters at 110–180 °C with yields for ethane of up to 60 % with over 90 % selectivity. Experimental and computational studies support a unique mechanism that involves Sb V ‐mediated C−H activation followed by functionalization of a Sb V ‐alkyl intermediate." @default.
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• W2907019107 date "2019-01-21" @default.
• W2907019107 modified "2023-10-03" @default.
• W2907019107 title "Selective C−H Functionalization of Methane and Ethane by a Molecular Sb ^V Complex" @default.
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• W2907019107 doi "https://doi.org/10.1002/anie.201809159" @default.
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