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- W2907278639 abstract "A family of Pd–IPr complexes (1Pd–6Pd) featuring electropositive and bulky R3Si substituents at the 4-position of the NHC ring was prepared and fully characterized. The catalytic performance of 1Pd (R3Si = SiMe3) and 3Pd (R3Si = Si(allyl)Me2) in the Buchwald–Hartwig amination was excellent, notably outperforming those of other previously reported catalytic systems by requiring shorter reaction times, lower catalyst loadings, and milder reaction conditions. Furthermore, a systematic evaluation of both the electronic and steric influences of the 4-R3Si-IPr ligand on the overall catalytic performance of 1Pd–6Pd revealed that electronic rather than steric factors play a dominant role." @default.
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- W2907278639 date "2018-12-31" @default.
- W2907278639 modified "2023-10-01" @default.
- W2907278639 title "[Pd(4-R<sub>3</sub>Si-IPr)(allyl)Cl], a Family of Silyl-Substituted Pd–NHC Complexes: Catalytic Systems for the Buchwald–Hartwig Amination" @default.
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- W2907278639 doi "https://doi.org/10.1021/acs.organomet.8b00757" @default.
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