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- W2907651631 abstract "A previously reported cobalt complex featuring a tetraimidazolyl-substituted pyridine chelate is an active water oxidation electrocatalyst with moderate overpotential at pH 7. While this complex decomposes rapidly to a less-active species under electrocatalytic conditions, detailed electrochemical studies support the agency of an initial molecular catalyst. Cyclic voltammetry measurements confirm that the imidazolyl donors result in a more electron-rich Co center when compared with previous pyridine-based systems. The primary changes in electrocatalytic behavior of the present case are enhanced activity at lower pH and a marked dependence of catalytic activity on pH." @default.
- W2907651631 created "2019-01-11" @default.
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- W2907651631 date "2018-12-27" @default.
- W2907651631 modified "2023-10-08" @default.
- W2907651631 title "Imidazole for Pyridine Substitution Leads to Enhanced Activity Under Milder Conditions in Cobalt Water Oxidation Electrocatalysis" @default.
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- W2907651631 doi "https://doi.org/10.1021/acs.inorgchem.8b02942" @default.
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